Preview

Proceedings of the National Academy of Sciences of Belarus. Physical-technical series

Advanced search

A SOURCE OF NEUTRON CAPTURE GAMMA-RAY WITH ENERGY TO 7 MeV AND TO 10 MeV BASED ON NEUTRON CALIBRATION FACILITY

Abstract

Wide spread of technogenic sources of ionizing radiation such as particle accelerators and nuclear reactors leads to appearance of a number of applied metrological tasks aimed at providing spectrometric and dosimetric ionization measurement instruments, located in photon radiation fields with energy to 10 MeV. Gamma rays with energy higher 3 MeV may be acquired using radioactive thermal neutron capture on target, i.e. (n, γ)-nuclear reaction. Titanium is used in the range of energies to 7 MeV; nickel – to 10 MeV. A simplest source of instantaneous neutron capture gamma-ray should consist of fast neutron source, neutron moderator and a target irradiated with thermal neutrons. The collimator with thermal neutron geometry of АТ140 neutron calibration facility with 238Pu–Be fast neutron source may be used (IBN–8–6) as a source of gamma-ray with energy to 10 MeV. Monte-Carlo models of thermal neutrons geometry, facility and 238Pu–Be fast neutron source were built using MCNP–4b code. Energy distribution of flux density of neutron capture gamma–ray for titanium and nickel targets was defined. A spectrometric detector based on LaBr3(Ce) crystal Ø 38×38 mm with non-linear characteristics of channel-energy transformation in the range up to 10 MeV, was specifically manufactured for instrumental support of the experiment at SPE “ATOMTEX”. The results for Ti, Ni, and for bare 238Pu–Be neutron source were acquired. During the experiment a possibility to use neutron capture gamma-ray field formed by thermal neutrons geometry of АТ140 neutron calibration facility with 238Pu–Be-fast neutron source with Ti and Ni targets for calibration LaBr3(Ce) spectrometers for energy to 10 MeV was confirmed. Closely stationing polyethylene plate in collimator channel provides significant increase in output of reference radiation from target simultaneously decreasing unneeded parts of the spectrum. 

About the Authors

D. I. Komar
SPE “ATOMTEX”
Belarus
engineer


R. V. Lukashevich
SPE “ATOMTEX”
Belarus
lead engineer


V. D. Guzov
SPE “ATOMTEX”
Belarus
Head of Metrology Department


S. A. Kutsen
Research Institute for Nuclear Problems of Belarusian State University
Belarus
Ph. D. (Physics and Mathematics), Head of Laboratory of theoretical physics and simulation of nuclear processes


References

1. Bermann F., Bordy J. M., Chassende-Baroz P., Detroussel P., Dhermain J., Jaureguy J. C., Sollier T. Capture Gamma Ray Beam for the Calibration of Radioprotection Dosemeters between 5 and 9 MeV. Radiation Protection Dosymetry, 1990, no. 4, pp. 237–243. Doi: 10.1093/oxfordjournals.rpd.a080623

2. International Electrotechnical Commission. Radiation Protection Instrumentation – Transportable, Mobile or Installed Equipment to Measure Photon Radiation for Environmental Monitoring. 23/10/2015 no. IEC 61017 Ed. 1.

3. International Standart “X and gamma radiation for calibrating dosimeters and dose rate meters and for determining their response as a function of photon energy”. 15/12/1996. ISO 4037-1.

4. Duvall K. C., Heaton H. T., Soares C. G. The development of a 6–7 MeV photon field for instrument calibration. Nuclear Instruments and Methods in Physics Research, 1985, vol. 10–11, no. 2, pp. 942–945. Doi: 10.1016/0168–583X(85)90145–4

5. Guldbakke S., Schaffer S. Properties of high-energy photon fields to be applied for calibration purposes. Nuclear Instruments and Metods in Physics Research, 1990, vol. 299, no. 1–3, pp. 367–371. Doi: 10.1016/0168–9002(90)90806–H

6. Rogers D. O. A nearly mono-energetic 6–7 MeV photon calibration source. Health Physics, 1983, vol. 45, no. 1, pp. 127–137. Doi: 10.1097/00004032–198307000–0001

7. Croft S., Bailey M. The determination of the adsolute responce function of a deuterated benzene total energy detector to 6,13 MeV γ-rays. Nuclear Instruments and Methods in Physics Research, 1991, vol. 302, no. 2, pp. 315–326. Doi: 10.1016/0168– 9002(91)90415–M

8. Bermann F. Étalonnage de détecteurs de radioprotection avec des gammas d’énergie supérieure à 1 MeV: utilisation de faisceaux de gammas de capture, Radioprotection, 1991, vol. 26, no. 3, pp. 493–513. Doi: 10.1051/radiopro/1991017

9. Kroupa M., Granja C., Janout Z. Wide energy range gamma-ray calibration source. Journal of Instrumentation, 2011, vol. 6, no. 1, pp. 6–11. Doi: 10.1088/1748–0221/6/11/T11002

10. Rogers J. G., Andreaco M. S., Moisan C. A 7–9 MeV isotopic gamma-ray source for detector testing. Nuclear Instruments and Metods in Physics Research, 1998, vol. 413, no. 2–3, pp. 249–254. Doi: 10.1016/S0168–9002(98)00097–7

11. Komar D., Lukashevich R., Guzov V., Kutsen S. Neutron capture gamma ray field with energy to 10 MeV for metro-logical support of radiation protection devices. Pribory i metody izmerenii [Devices and Methods of Measurements], 2016, vol. 7, no. 3, pp. 296–304. Doi: 10.21122/2220–9506–2016–7–3–296–304 (in Russian).

12. Briestmeister J. F. [ed.]. MCNP-A general Monte Carlo N-particle transport code, Version 4A. Report LA–12625–M. Los Alamos, NM, Los Alamos National Laboratory, 1994. 736 p.

13. Komar D. I., Kutsen S. A., Guzov V. D. Monte-Carlo simulation metrological characteristics of the neutron calibration facility. Ekologicheskij vestnik [Ecological proceedings], 2016, no. 3, pp. 54–61 (in Russian).

14. Komar D., Kutsen S. Influence of scattered neutron radiation on metrological characterictics of AT140 Neutron Calibration Facility. Pribory i metody izmerenii [Devices and Methods of Measurements], 2017, vol. 8, no. 1, pp. 23–31. Doi: 10.21122/2220– 9506–2017–8–1–23–31 (in Russian).

15. Choi H. D., Firestone R. B., Lindstorm R. B. Database of promt gamma-rays from slow neutron capture for elemental analysis. Vienna, International Atomic Energy Agency, 2006. 252 p.

16. Kopecky, J. [ed.] Atlas of Neutron Capture Cross Sections. Vienna, International Atomic Energy Agency, 1997. 370 p.

17. Ceberg C. P., Salford L. G. Neutron capture imaging of 10B in tissue specimens. Radiotherapy and Oncology, 1993, vol. 26, no. 2, pp. 139–146. Doi: 10.1016/0167–8140(93)90095–P

18. Hugh E. H. Neutron Inelastic Scattering in 12C, 14N and 16O. Houston, Texas, 1959. 256 p.

19. Baldini A., Bemporad C., Cei F. A NaI activation method for the measurement of the weak thermal neutron field around the MEG experiment. Nuclear Instruments and Methods in Physics Research, 2007, vol. 570, no. 3, pp. 561–564. Doi: 10.1016/j.nima.2006.10.101

20. Gardner R. P., Sayyed E., Zheng Y. NaI detector neutron activation spectra for PGNAA applications. Applied Radiation and Isotopes, 2000, vol. 53, no. 4–5, pp. 483–497. Doi: 10.1016/S0969–8043(00)00198–6


Review

Views: 756


Creative Commons License
This work is licensed under a Creative Commons Attribution 4.0 License.


ISSN 1561-8358 (Print)
ISSN 2524-244X (Online)